期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 57, 期 46, 页码 15086-15090出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201808242
关键词
chemiresistive sensing; electrical conductivity; metal-organic frameworks; molecular devices; ultrathin films
资金
- EU [ERC Stg Chem-fs-MOF 714122, SPIN2D H2020/2014-659378]
- Spanish MINECO [MDM-2015-0538, RYC-2012-10894]
- Spanish MECD [FPU13/03203]
- Generalitat Valenciana [GRISOLIA/2015/007]
Conductive metal-organic frameworks are opening new perspectives for the use of these porous materials for applications traditionally limited to more classical inorganic materials, such as their integration into electronic devices. This has enabled the development of chemiresistive sensors capable of transducing the presence of specific guests into an electrical response with good selectivity and sensitivity. By combining experimental data with computational modelling, a possible origin for the underlying mechanism of this phenomenon in ultrathin films (ca.30 nm) of Cu-CAT-1 is described.
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