期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 14, 页码 3552-3557出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201309253
关键词
boranes; frustrated Lewis pairs; hydrogenation; metathesis; olefins
资金
- German Science Foundation (DFG)
The metal-free activation of hydrogen by frustrated Lewis pairs (FLPs) is a valuable method for the hydrogenation of polarized unsaturated molecules ranging from imines, enamines, and silyl enol ethers to heterocycles. However, one of the most important applications of hydrogenation technology is the conversion of unsaturated hydrocarbons into alkanes or alkenes. Despite the fast development of the FLP chemistry, such reactions proved as highly challenging. This Minireview provides an overview of the basic concepts of FLP chemistry, the challenge in the hydrogenation of unsaturated hydrocarbons, and first solutions to this central transformation.
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