期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 33, 页码 8634-8639出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201403747
关键词
biorefinery; catalytic hydrogen transfer; cellulose; enzymatic hydrolysis; lignin
资金
- Alexander von Humboldt Foundation
- German Federal government
- German State government
- Max Planck-Fraunhofer Cooperation Scheme
Through catalytic hydrogen transfer reactions, a new biorefining method results in the isolation of depolymerized lignin-a non-pyrolytic lignin bio-oil-in addition to pulps that are amenable to enzymatic hydrolysis. Compared with organosolv lignin, the lignin bio-oil is highly susceptible to further hydrodeoxygenation under low-severity conditions and therefore establishes a unique platform for lignin valorization by heterogeneous catalysis. Overall, the potential of a catalytic biorefining method designed from the perspective of lignin utilization is reported.
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