期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 28, 页码 7281-7285出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201403946
关键词
carbon; electrocatalysis; nanostructures; oxygen evolution; porous structure
资金
- Australian Research Council (ARC) [DP140104062, DP130104459]
A new class of highly efficient oxygen evolution catalysts has been synthesized through the self-assembly of graphitic carbon nitride nanosheets and carbon nanotubes, driven by pi-pi stacking and electrostatic interactions. Remarkably, the catalysts exhibit higher catalytic oxygen evolution activity and stronger durability than Ir-based noble-metal catalysts and display the best performance among the reported nonmetal catalysts. This good result is attributed to the high nitrogen content and the efficient mass and charge transfer in the porous three-dimensional nanostructure.
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