期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 14, 页码 3684-3687出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201310562
关键词
axial chirality; BINAM; Bronsted acids; enantioselectivity; kinetic resolution
资金
- National Natural Science Foundation of China [21232007, 21302088, 21302087]
- National Basic Research Program of China (973 Program) [2010CB833300]
- Shenzhen special funds for the development of biomedicine, Internet, new energy, and new material industries [JCYJ20130401144532131, JCYJ20130401144532137]
- South University of Science and Technology of China
A highly efficient strategy for the kinetic resolution of axially chiral BINAM derivatives involving a chiral Bronsted acid-catalyzed imine formation and transfer hydrogenation cascade process was developed. The kinetic resolution provides a convenient route to chiral BINAM derivatives in high yields with excellent enantioselectivities.
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