期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 42, 页码 11285-11288出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201405647
关键词
aldehydes; C-H activation; chemoselectivity; oxygenation; ruthenium
资金
- European Research Council under the European Community [307535]
- CaSuS program
- Chinese Scholarship Program
Versatile ruthenium(II) complexes allow for site-selective CH oxygenations with weakly-coordinating aldehydes. The challenging CH functionalizations proceed with high chemoselectivity by rate-determining CH metalation. The new method features an ample substrate scope, which sets the stage for the step-economical preparation of various bioactive heterocycles.
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