期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 10, 页码 2648-2653出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201309718
关键词
colloids; gold nanorods; palladium nanorods; plasmonic polymers; step-growth copolymerization
资金
- Canada Research Chair
- Ontario Ministry of Economic Development and Innovation
- NSERC Canada through a BiopSys Strategic Network Grant
- 1000 Young Talent Plan of China
- Jilin University
- National Science Foundation [DMR-1309892, DMR-1121107, DMR-1122483]
- National Institutes of Health [P01-HL108808]
- Cystic Fibrosis Foundation
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1309892] Funding Source: National Science Foundation
The resemblance between colloidal and molecular polymerization reactions is very useful in fundamental studies of polymerization reactions, as well as in the development of new nanoscale systems with desired properties. Future applications of colloidal polymers will require nanoparticle ensembles with a high degree of complexity that can be realized by hetero-assembly of NPs with different dimensions, shapes, and compositions. A method has been developed to apply strategies from molecular copolymerization to the co-assembly of gold nanorods with different dimensions into random and block copolymer structures (plasmonic copolymers). The approach was extended to the co-assembly of random copolymers of gold and palladium nanorods. A kinetic model validated and further expanded the kinetic theories developed for molecular copolymerization reactions.
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