期刊
JETP LETTERS
卷 85, 期 3, 页码 174-178出版社
MAIK NAUKA/INTERPERIODICA/SPRINGER
DOI: 10.1134/S0021364007030095
关键词
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Conduction-electron spin polarization dynamics achieved by pulsed optical pumping at room temperature in GaAs1-xNx alloys with a small nitrogen content (x = 2.1, 2.7, and 3.4%) is studied both experimentally and GaAs, theoretically. It is found that the photoluminescence circular polarization determined by the mean spin of free electrons reaches 40-45% and this giant value persists within 2 ns. Simultaneously, the total free-electron spin decays rapidly with the characteristic time approximate to 150 ps. The results are explained by spin-dependent capture of free conduction electrons on deep paramagnetic centers resulting in the dynamical polarization of bound electrons. A nonlinear theory of spin dynamics in the coupled system of spin-polarized free and localized carriers has been developed which describes the experimental dependencies, in particular, the electron spin quantum beats observed in a transverse magnetic field.
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