期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 43, 页码 11463-11466出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201405131
关键词
anion; lanthanide; rotaxane; supramolecular chemistry; template synthesis
资金
- EPSRC
- European Research Council under the European Union [267426]
The first anion-templated synthesis of a lanthanide-containing interlocked molecule is demonstrated by utilizing a nitrite anion to template initial pseudorotaxane formation. Subsequent stoppering of the interpenetrated assembly allows for the preparation of a lanthanide-functionalized [2]rotaxane in high yield. Following removal of the nitrite anion template, the europium [2]rotaxane host is demonstrated to recognize and sense fluoride selectively.
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