期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 40, 页码 10763-10767出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201406098
关键词
C-H activation; carbenoids; multicomponent reactions; natural products; ruthenium
资金
- NSFC [21232007]
- MOST [2010CB833300]
- Ministry of Education
- CAS
A combination of either ruthenium(II) or rhodium(II) complexes and quinine-derived squaramide enables 3-diazooxindoles, indoles, and nitroalkenes to undergo highly efficient asymmetric three-component reactions, thus affording optically active 3,3'-bis(indole)s through a consecutive C-C bond-forming sequence, which turned out to be applicable to the facile total synthesis of (-)-folicanthine.
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