期刊
JOURNAL OF COLLOID AND INTERFACE SCIENCE
卷 306, 期 2, 页码 255-261出版社
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcis.2006.10.078
关键词
tetrahydrofuran clathrate hydrate; particle adhesion; micromechanical testing; capillary bridging; sorbitan monolaurate (Span20); poly-N-vinyl caprolactam (PVCap)
Adhesion forces between tetrahydrofuran (THF) hydrate particles in n-decane were measured using an improved micromechanical technique. The experiments were performed at atmospheric pressure over the temperature range 261-275 K. The observed forces and trends were explained by a capillary bridge between the particles. The adhesion force of hydrates was directly proportional to the contact force and contact time. A scoping study examined the effects of temperature, anti-agglomerants, and interfacial energy on the particle adhesion forces. The adhesion force of hydrates was found to be directly proportional to interfacial energy of the Surrounding liquid, and to increase with temperature. Both sorbitan monolaurate (Span20) and poly-N-vinyl caprolactam (PVCap) decreased the adhesion force between the hydrate particles. (c) 2006 Elsevier Inc. All rights reserved.
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