期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 53, 期 35, 页码 9298-9301出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201311124
关键词
carbon dioxide capture/release; diarylethene ligands; metal-organic frameworks; photochromism; photoswitching
资金
- 973 Program [2011CBA00505]
- NSF of China [21203022, 21261001, 21221001]
- NSF of Fujian Province [2011J06006]
- Foundation of Jiangxi Educational Committee [GJJ13472]
We demonstrate herein a promising pathway towards low-energy CO2 capture and release triggered by UV and visible light. A photosensitive diarylethene ligand was used to construct a photochromic diarylethene metal-organic framework (DMOF). A local photochromic reaction originating from the framework movement induced by the photoswitchable diarylethene unit resulted in record CO2-desorption capacity of 75% under static irradiation and 76% under dynamic irradiation.
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