期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 129, 期 8, 页码 2230-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja068886f
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资金
- NIGMS NIH HHS [R01 GM065865, R01 GM065865-04, R01GM065865] Funding Source: Medline
We report an intermolecular oxidative coupling of alkynamides and terminal alkenes to synthesize E-alpha,beta-unsaturated ketones under very mild conditions using catalytic Pd(II) and an oxidant. An O-17 isotope labeling experiment implicates a cyclic oxypalladation intermediate in this reaction.
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