The authors present partial-ion-yield experiments on the methyl chloride molecule excited in the vicinity of the C12p and C1s inner shells. A large number of fragments, cations produced by dissociation or recombination processes, as well as anionic species, have been detected. Although the spectra exhibit different intensity distributions depending on the core-excited atom, general observations include strong site-selective fragmentation along the C-Cl bond axis and a strong intensity dependence of transitions involving Rydberg series on fragment size. (c) 2007 American Institute of Physics.
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