期刊
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
卷 2007, 期 10, 页码 1599-1605出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.200600945
关键词
annulation; homogeneous catalysis; hydrogen transfer; ruthenium; synthetic methods
The first synthesis of polysubstituted quinoline derivatives from aromatic or aliphatic alcohols with RuCl2(dmso)(4) as catalyst under solvent-free conditions is described. The reaction involves the in situ oxidation of alcohols to the corresponding carbonyl compounds through a hydrogen-transfer, followed by a Friedlander annulation process. The whole process is a mild, efficient, selective, and high-yielding single-step procedure. ((c) Wiley-VCH Verlag GmbH & Co.
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