Quasi-phase-matched second-harmonic generation of 532 nm radiation in 25 degrees-rotated, x-cut, near-stoichiometric lithium tantalate has been performed. Using a face-normal topology for frequency conversion applications allows scalable surface area to avoid surface and volume damage in high-power interactions. First-order, quasi-phase-matched second-harmonic generation was achieved using near-stoichiometric lithium tantalate fabricated by vapor transport equilibration. These crystals supported 1 J of 1064 nm radiation and generated 21 mJ of 532 ma radiation from a 7 ns, Q-switched Nd: YAG laser within a factor of 4.2 of expectation. (c) 2007 Optical Society of America.
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