期刊
JOURNAL OF PHYSICS-CONDENSED MATTER
卷 19, 期 17, 页码 -出版社
IOP PUBLISHING LTD
DOI: 10.1088/0953-8984/19/17/176229
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We report experimentally that room-temperature ferromagnetism of Co-doped ZnO is strongly correlated with structural defects, and that carriers involved in carrier-mediated exchange are by nature by-products of the creation of the defects. On the other hand, the carrier concentration has pronounced influences on the absorption edge in optical transmission spectra of epitaxial Co: ZnO films, in which both a blue-shift and a red-shift are observed. Furthermore, high-temperature annealing results in evolution of the local Co structure from Co2+ replacing Zn2+ to a Co3O4-based phase, which most likely accounts for the transition from ferromagnetism to paramagnetism in the Co:ZnO films.
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