Quantum projection in an ising spin liquid

A transverse magnetic field is used to scan the diagonal and off-diagonal susceptibility of the uniaxial quantum magnet, LiHo0.045Y0.955F4. Clusters of strongly coupled spins act as the primary source for the response functions, which result from a field-induced quantum projection of the system into a classically forbidden (meaning non-Ising) regime. Calculations based on spin pairs reproduce only some features of the data and fail to predict the measured off-diagonal response, providing evidence of a multispin collective state.