期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 129, 期 33, 页码 10096-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja073912a
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We describe a single-step conversion of various N-vinyl and N-aryl amides to the corresponding pyridine and quinoline derivatives, respectively. The process involves amide activation with trifluoromethanesulfonic anhydride in the presence of 2-chloropyridine followed by pi-nucleophile addition to the activated intermediate and annulation. Compatibility of this chemistry with sensitive N-vinyl amides, epimerizable substrates, and a variety of functional groups is noteworthy.
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