期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 129, 期 36, 页码 11033-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja0724792
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Here we describe an approach that directly and unambiguously establishes the synergistic effect between surfaces when brought into close proximity (angstrom's regime) through the use of a scanning tunneling microscope. As a model system, we have employed the electrocatalytic oxidation of CO chemisorbed onto a Pt(111) single-crystal electrode upon engaging a Ru tip. Not only have we been able to observe clear and compelling evidence of a synergistic effect, but also, this approach provides valuable mechanistic details not accessible from conventional measurements.
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