期刊
CHEMICAL PHYSICS LETTERS
卷 446, 期 1-3, 页码 20-24出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.cplett.2007.08.040
关键词
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One of the key questions underlying adenine's photochemistry following 266 nm excitation is whether or not the dissociative (1)pi sigma* state plays an active role in the ensuing dynamics. This work describes how laser fluence studies on the Ad(+) and H+ following photo-excitation using a combination of ns and fs UY pulses with time-of-flight mass-spectrometry, provides new evidence that implicates the contentious participation of the (1)pi sigma* state in the photochemistry of adenine. (C) 2007 Elsevier B.V. All rights reserved.
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