期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 129, 期 41, 页码 12398-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja0753389
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资金
- NIGMS NIH HHS [GM13598, R01 GM013598-43, R01 GM013598] Funding Source: Medline
The transition metal-catalyzed trimethylenemethane [3+2] cycloaddition provides a direct route to functionalized heterocycles. Herein, we describe a catalytic, asymmetric protocol for the reaction between 3-acetoxy-2-trimethylsilylmethyl-l-propene and various imines. The corresponding pyrrolidines were obtained in excellent yields and enantioselectivities making use of the novel phosphoramidite L10.
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