期刊
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS
卷 40, 期 20, 页码 F285-F291出版社
IOP PUBLISHING LTD
DOI: 10.1088/0953-4075/40/20/F01
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Angular distributions of C 1s photoelectrons, relative to a dissociation axis for C2H2, have been measured with a photoelectron - photoion - photoion coincidence technique. The photoelectron angular distribution ( PAD) for three two- body fragmentations ( symmetric, non- symmetric and proton- migration fragmentations) is completely different. The PADs for non- symmetric fragmentation provide direct evidence of a localized core- hole and preferential bond breaking following Auger decays. Moreover, the PAD for symmetric fragmentation has been interpreted as the interference between photoemissions from the two carbon atoms.
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