期刊
PHYSICAL REVIEW LETTERS
卷 99, 期 18, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.99.183902
关键词
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The response of the electronic system of LiH to a few-cycle strong field is computed by a time-dependent multiconfiguration method using a large, adaptive, basis set. The intensity, pulse duration, polarization, and phase of carrier frequency can all be tuned to steer the motion of the electrons. It is shown possible to, e.g., direct the electrons to move along the Li-H bond or normal to it. By shifting the phase, the electrons can be driven toward the Li nucleus or away from it. When the pulse is polarized not along the bond the result is a rotation of the charge density.
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