期刊
CURRENT OPINION IN COLLOID & INTERFACE SCIENCE
卷 12, 期 6, 页码 285-296出版社
ELSEVIER SCIENCE LONDON
DOI: 10.1016/j.cocis.2007.08.014
关键词
single molecule fluorescence; Markov process; hidden Markov models; reaction rate theory; molecular memory
资金
- NIGMS NIH HHS [R01 GM071684-04, R01 GM071684-01, R01 GM071684-02, R01 GM071684-03, R01 GM071684] Funding Source: Medline
This article examines the current status of Markov processes in single molecule fluorescence. For molecular dynamics to be described by a Markov process, the Markov process must include all states involved in the dynamics and the first-passage time (FPT) distributions out of those states must be describable by a simple exponential law. The observation of non-exponential FPT distributions or other evidence of non-Markovian dynamics is common in single molecule studies and offers an opportunity to expand the Markov model to include new dynamics or states that improve understanding of the system. (c) 2007 Elsevier Ltd. All rights reserved.
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