期刊
AICHE JOURNAL
卷 59, 期 10, 页码 3574-3577出版社
WILEY-BLACKWELL
DOI: 10.1002/aic.14208
关键词
catalysis; adsorption; activity distribution; simulation; transient response; temporal analysis of products
资金
- National Science and Technology Development Agency
- Crown Property Bureau under the National Science and Technology Development Agency
- NANOTEC Center of Excellence
- National Nanotechnology Center
- Thailand Research Fund (TRF)
- Commission on Higher Education, Ministry of Education
- National Research University Project of Thailand (NRU)
- National Center for Petroleum, Petrochemical and Advanced Materials (PPAM)
- Kasetsart University Research and Development Institute (KURDI)
- Ghent University [BOF/GOA 01GA0405]
- Flemish Government
Significance The described computational experiment focuses on producing a controlled catalyst activity distribution. Using TAP technique, the activity profile on the solid catalytic material surface is created by adsorption of pulsed feed gas or the like process and is controlled by the total amount of pulsed gas following the coincidence property. The coincidence property is also applicable for other diffusion+irreversible adsorption processes like wet impregnation to prepare catalyst with nonuniform distribution of catalytic material. (c) 2013 American Institute of Chemical Engineers AIChE J, 59: 3574-3577, 2013
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