期刊
AEROSOL SCIENCE AND TECHNOLOGY
卷 42, 期 10, 页码 862-871出版社
TAYLOR & FRANCIS INC
DOI: 10.1080/02786820802339579
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资金
- Office of Science (BER), U.S. Department of Energy [DE-GF02-05ER63997]
- National Science Foundation Award [ATM0506674]
- California Air Resources Board ICAT program [04-03]
An ultrafine, water-based condensation particle counter (U-WCPC, TSI Model 3786) has been compared to a butanol-based ultrafine counter (U-BCPC, TSI Model 3025) for measurement of atmospheric and freeway-tunnel aerosols. The U-WCPC utilizes a warm, wet-walled growth tube to activate and grow particles through water condensation in a laminar-flow. It has an aerosol sampling rate of 0.3 L/min, and a nominal detection limit near 3 nm. Several field comparisons were made to the butanol-based instrument with the same nominal detection limit. For measurements of size-selected aerosols with diameters of 5 nm and larger the two instruments generally agreed, with a mean response within 5%. At 3 nm particle size differences were observed, and these differences varied with the data set. Measurements of ambient aerosol in Boulder, Colorado showed higher counting efficiency at 3 nm with the U-BCPC, while in a California freeway tunnel the opposite trend was observed, with higher counting efficiencies at 3 nm observed by the U-WCPC. For direct measurement of atmospheric aerosols, the two types of instruments yielded equivalent concentrations, independent of particle number concentration.
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