期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 360, 期 24, 页码 4774-4783出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201801058
关键词
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资金
- National Natural Science Foundation of China [NSFC-21572178, NSFC-21702162]
- Natural Science Basic Research Plan in Shaanxi Province of China [2017JM2006]
- Key Science and Technology Innovation Team of Shaanxi Province [2017KCT-37]
- Scientific Research Program - Shaanxi Provincial Education Department [17JK0788]
A general, efficient and economic palladium-catalyzed dehydrogenation to form enones or enals has been developed. The approach possesses extremely broad substrate scope including various linear or cyclic saturated ketones and aldehydes. The protocol is ligand-free, and molecular oxygen is used as the sole clean oxidant in the reaction. Due to mild reaction conditions, good functional group compatibility, and versatile utilities of enones and enals, the method can be applied in the late-stage synthesis of natural products, pharmaceuticals and fine chemicals.
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