期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 353, 期 16, 页码 2988-2998出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201100362
关键词
C?H activation; heterogeneous catalysis; nanomaterials; palladium; polyoxometalates
资金
- Institute of Bioengineering and Nanotechnology (Biomedical Research Council, Agency for Science, Technology and Research, Singapore)
An efficient heterogeneous palladium-polyoxometalate catalyst with the formula Pd-H6PV3Mo9O40/C has been successfully developed for carbon-carbon (C?C) bond formation via carbon-hydrogen (C?H) activation and carbon-nitrogen (C?N) bond formation via oxidative amination using oxygen as the terminal oxidant. The coupling processes are simple, and use relatively mild conditions to form the desired products. In addition, less waste is generated as no additional reagents such as organic/inorganic oxidants are required, and water is the only by-product generated.
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