期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 353, 期 18, 页码 3373-3379出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201100417
关键词
acylation; benzylic alcohols; oxidative C?H activation; palladium catalysis; triflic acid
资金
- National Natural Science Foundation of China [20702043]
- Yangzhou University
- Priority Academic Program Development of Jiangsu Higher Education Institutions
An efficient and clean method to construct C?C bonds has been developed via the acylation reaction of acetanilides with benzylic alcohols using tert-butyl hydroperoxide (TBHP) as oxidant catalyzed by palladium acetate in the presence of triflic acid (TfOH). The acylation reactions exhibit excellent reactivities, and up to 95% yield of the corresponding aryl ketone could be obtained under the optimal conditions.
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