期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 351, 期 9, 页码 1390-1394出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.200800815
关键词
heterogeneous catalysis; hydrosilylation; N-heterocyclic carbenes; organocatalysis
资金
- Institute of Bioengineering and Nanotechnology (Biomedical Research Council, Agency for Science, Technology and Research, Singapore)
N-Heterocyclic carbene (NHC)-catalyzed ketone/imine hydrosilylation, silane alcohol condensation and asymmetric ketone hydrosilylation reactions were demonstrated for the first time over solid, main-chain poly-NHC particles. The stable and robust poly-NHC particles were easily recovered, and exhibited good catalytic recyclability. A novel chiral induction protocol with a cheap and easily accessible secondary alcohol as the chiral source was also developed in this catalytic system.
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