期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 350, 期 10, 页码 1526-1530出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.200800157
关键词
cycloaddition; hypervalent compounds; imines; methylene compounds; nitrogen heterocycles; oxidation
Aziridination of N-tosylimines with activated methylene compounds induced by iodobenzene diacetate [PhI(OAc)(2)] and tetrabutylammonium bromide [Bu4NBr] afforded the corresponding 2,2-difunctionalized aziridines in good yields with the aid of a catalytic amount of base. The reaction is hypothesized to proceed via a tandem nucleophilic addition-oxidative cyclization pathway.
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