期刊
ADVANCED MATERIALS
卷 22, 期 9, 页码 951-+出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.200902039
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资金
- National Natural Science Foundation of China [50972090]
- Program for New Century Excellent Talents in university [NCET-04-0387]
- National Basic Research Program of China [2006CB601200]
- Major Fundamental Research Project of Shanghai Science Committee [07DJ14001]
- Dawn program of Shanghai Education Commission [08SG15]
Artificial inorganic leafs are developed by organizing light harvesting, photoinduced charge separation, and catalysis modules (Pt/N-TiO2) into leaf-shaped hierarchical structures using natural leaves as biotemplates (see figure). The enhanced light-harvesting and photocatalytic water-splitting activities stem from the reproduction of the leafs' complex structures and self-doping of nitrogen during synthesis. The research may represent an important first step toward the design of novel artificial solar-energy transduction systems based on natural concepts, particularly on mimicking the structural design.
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