期刊
ADVANCED FUNCTIONAL MATERIALS
卷 23, 期 21, 页码 2775-2781出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201202956
关键词
dye-sensitized solar cell; titanium dioxide; atomic layer deposition; cobalt complex; templates
类别
资金
- EU [NMP-229036]
- Center for Advanced Molecular Photovoltaics, King Abdullah University of Science and Technology (KAUST) [KUS-C1-015-21]
- Balzan foundation
- Ministry of Education, Science and Technology through the National Research Foundation of Korea [R31-2008-000-10035-0]
In this paper, a way of utilizing thin and conformal overlayer of titanium dioxide on an insulating mesoporous template as a photoanode for dye-sensitized solar cells is presented. Different thicknesses of TiO2 ranging from 1 to 15 nm are deposited on the surface of the template by atomic layer deposition. This systematic study helps unraveling the minimum critical thickness of the TiO2 overlayer required to transport the photogenerated electrons efficiently. A merely 6-nm-thick TiO2 film on a 3-m mesoporous insulating substrate is shown to transport 8 mA/cm2 of photocurrent density along with approximate to 900 mV of open-circuit potential when using our standard donor--acceptor sensitizer and Co(bipyridine) redox mediator.
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