期刊
ADVANCED FUNCTIONAL MATERIALS
卷 24, 期 9, 页码 1284-1289出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201302169
关键词
lithium sulfur batteries; electrochemistry; sulfur utilization; electrode materials; cycle stability
The lithium sulfur battery system has been studied since the late 1970s and has seen renewed interest in recent years. However, even after three decades of intensive research, prolonged cycling can only be achieved when a large excess of electrolyte and lithium is used. Here, for the first time, a balanced and stable lithium sulfur fullcell is demonstrated with silicon-carbon as well as all-carbon anodes. More than 1000 cycles, a specific capacity up to 1470 mAh g(-1) (sulfur) (720 mAh g(-1) (cathode)), and a high coulombic efficiency of over 99% even with a low amount of electrolyte are achieved. The alternative anodes do not suffer from electrolyte depletion, which is found to be the main cause of cell failure when using metallic lithium anodes.
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