期刊
ADVANCED FUNCTIONAL MATERIALS
卷 22, 期 12, 页码 2594-2605出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201102622
关键词
bulk heterojunctions; solar cells; metal oxides; hole transport; MoOx
类别
资金
- Department of Energy (DOE) [DE-FG02-08ER46535]
- NSF [DMR-1121053]
- CSIRO, Australian Research Council [DP110105341]
- Australian Solar Institute USASEC
- Fulbright Postdoctoral Fellowship Scheme
- U.S. Department of Energy (DOE) [DE-FG02-08ER46535] Funding Source: U.S. Department of Energy (DOE)
A simple, solution-processed route to the development of MoOx thin-films using oxomolybdate precursors is presented. The chemical, structural, and electronic properties of these species are characterized in detail, within solution and thin-films, using electrospray ionization mass spectrometry, grazing angle Fourier transform infrared spectroscopy, thermogravimetric analysis, atomic force microscopy, X-ray photoelectron spectroscopy, and ultraviolet photoelectron spectroscopy. These analyses show that under suitable deposition conditions the resulting solution processed MoOx thin-films possess the appropriate morphological and electronic properties to be suitable for use in organic electronics. This is exemplified through the fabrication of poly(3-hexylthiophene):[6,6]-phenyl C61 butyric acid methyl ester (P3HT:PC61BM) bulk heterojunction (BHJ) solar cells and comparisons to the traditionally used poly(3,4-ethyldioxythiophene)/poly(styrenesulfonate) anode modifying layer.
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