期刊
ACS NANO
卷 7, 期 4, 页码 3598-3606出版社
AMER CHEMICAL SOC
DOI: 10.1021/nn400576v
关键词
electrochemical exfoliation; high-quality graphene; solution processing; organic field-effect transistors
类别
资金
- ERC grant on NANOGRAPH
- ERC grant on 2DMATER
- DFG Priority Program [SPP 1459]
- BMBF Graphenoid Project
- ESF Project GOSPEL [09-EuroGRAPHENE-FP-001]
- EU Project GENIUS
- EU Project MOLESOL
Solution-processable thin layer graphene is an intriguing nanomaterial with tremendous potential for electronic applications. In this work, we demonstrate that electrochemical exfoliation of graphite furnishes graphene sheets of high quality. The electrochemically exfoliated graphene (EG) contains a high yield (>80%) of one- to three-layer graphene flakes with high C/O ratio of 12.3 and low sheet resistance (4.8 k Omega/square for a single EG sheet). Due to the solution processability of EG, a vacuum filtration method in association with dry transfer is introduced to produce large-area and highly conductive graphene films on various substrates. Moreover, we demonstrate that the patterned EG can serve as high-performance source/drain electrodes for organic field-effect transistors.
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