4.8 Article

Fano Resonant Ring/Disk Plasmonic Nanocavities on Conducting Substrates for Advanced Biosensing

期刊

ACS NANO
卷 6, 期 11, 页码 9989-9995

出版社

AMER CHEMICAL SOC
DOI: 10.1021/nn303643w

关键词

plasmonics; Fano interference; ultrasensitive biosensing; figure of merit; refractive index sensitivity; nanocavities; nanofabrication

资金

  1. National Science Foundation (NSF) [ECCS-0954790]
  2. ONR [11PR00755-00-P00001]
  3. NSF Engineering Research Center on Smart Lighting [EEC-0812056]

向作者/读者索取更多资源

By introducing a conducting metal layer underneath a Fang resonant asymmetric ring/disk plasmonic nanocavity system, we demonstrate that electromagnetic fields. can be strongly enhanced. These large electromagnetic fields extending deep into the medium are highly accessible and increase the interaction volume of analytes and optical fields. As a result, we demonstrate high refractive Index sensitivities as large as 648 nm/RIU. By exciting Fano resonances with much sharper spectral features, as narrow as 9 nm, we experimentally show high figure of merits as large as 72 and reliable detection of protein mono- and bilayers. Furthermore, the conducting substrate enables strong interaction between fundamental and higher order modes of the system by minor structural asymmetries. This is very advantageous for experimental realization of systems supporting resonances with well-defined Fano-like line shape without requiring challenging fabrication resolution. Exploiting conducting metallic substrates and the associated propagating surface plasmons at their interface could be extended to other Fano resonant cavity geometries for improved biosensing performance.

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