期刊
ACS NANO
卷 5, 期 9, 页码 7662-7668出版社
AMER CHEMICAL SOC
DOI: 10.1021/nn202910t
关键词
quasi-free-standing graphene; silicon carbide; fluorine intercalation; scanning tunneling microscopy and spectroscopy; electronic structure; nanostructures
类别
资金
- NRF-CRP [R-143-000-360-281]
- NUS [R143-000-452-101]
- NUS Graduate School for Integrative Sciences and Engineering
We demonstrated a novel method to obtain charge neutral quasi-free-standing graphene on SIC (0001) from the buffer layer using fluorine from a molecular source, fluorinated fullerene (C60F48). The intercalated product is stable under ambient conditions and resistant to elevated temperatures of up to 1200 degrees C. Sunning tunneling microscopy and spectroscopy measurements are performed for the first time on such quasi-free-standing graphene to elucidate changes in the electronic and structural properties of both the graphene and interfacial layer. Novel structures due to a highly localized perturbation caused by the presence of adsorbed fluorine were produced in the intercalation process and investigated. Photoemission spectroscopy is used to confirm these electronic and structural changes.
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