期刊
ACS APPLIED MATERIALS & INTERFACES
卷 5, 期 5, 页码 1630-1635出版社
AMER CHEMICAL SOC
DOI: 10.1021/am3023724
关键词
vanadium dioxide; particulate film; self-assembly; porous film; optical controllability
资金
- National 973 Program of China [2009CB939903]
- NSF of China [91122034]
- NSF for Distinguished Young Scholars of China [51125006]
- NSF of Shanghai Grant [51121064]
- Innovation Program of the CAS [KJCX2-EW-W11]
- CAS/SAFEA International Partnership Program
Nanoparticle-assembled vanadium dioxide (VO2) films have been easily prepared with the assistance of cetyltrimethylammonium vanadate (CTAV) precursor which exhibits self-assembly properties. The obtained VO2 film has a micro/nano hierarchical porous structure, so its visible-light transmittance is significantly improved (similar to 25% increased compared to continuous film). The VO2 particle density as well as the film porosity can be facilely controlled by adjusting experimental parameters such as dip-coating speed. Accordingly, film optical properties can also be tuned to a large extent, in particular the visible transmittance (T-vis) and near infrared switching efficiency (Delta T-nir). These VO2 nanoparticle-assembled films prepared by this novel method provide a useful model to research the balance between T-vis and Delta T-nir.
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