期刊
ACS APPLIED MATERIALS & INTERFACES
卷 2, 期 1, 页码 7-10出版社
AMER CHEMICAL SOC
DOI: 10.1021/am900647h
关键词
Boolean logic; monolayers; thin films; sensors; communication
资金
- Helen and Martin Kimmel Center for Molecular Design
- Yeda-Sela Center for Basic Research
- Israel Science Foundation
- EU
Signal amplification has been demonstrated with surface-bound electrochromic complexes that can exist in one of two oxidation states (M2+/3+). Reaction of FeCl3 with covalently immobilized Os2+ complexes on glass substrates converts the metal centers. from one oxidation state to the other. The formed Fe2+ reduces a series of Ru3+-based monolayers. The absorption of light is coupled with the oxidation state of the complexes and provides the Output for the monolayer-based device. The gain of the setup can be controlled by the addition of a Fe2+ chelating ligand.
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