期刊
ORGANIC CHEMISTRY FRONTIERS
卷 5, 期 3, 页码 366-370出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7qo00866j
关键词
-
资金
- National Natural Science Foundation of China [21672037, 21532001]
Sulfonylative C-H bond functionalization through a copper-catalyzed three-component reaction of 8-aminoquinoline amides, DABCO center dot(SO2)(2) and aryldiazonium tetrafluoroborates is developed. Excellent selectivity in the para-position is observed for this copper-catalyzed transformation. This reaction is triggered by a copper-chelated complex via the coordination of the copper catalyst with the substrate and arylsulfonyl radical generated in situ, thus providing 5-sulfonyl-8-aminoquinoline amides in moderate to good yields.
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