期刊
RSC ADVANCES
卷 8, 期 28, 页码 15444-15447出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ra02009d
关键词
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资金
- NSFC [21572087, 21632003]
- Key program of Gansu province [17ZD2GC011]
- 111 program from the MOE of P. R. China
A C-1-symmetric N-heterocyclic carbene (NHC)-catalysed activation of isatin-derived enals under oxidative conditions was achieved. The in situ generated alpha,beta-unsaturated acyl azolium species was efficiently trapped by 1,3-dicarbonyl compounds via a Michael addition/spiroannualtion cascade, delivering a series of synthetically important spirooxindole delta-lactones with up to 96% enantioselectivity.
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