期刊
CATALYSIS SCIENCE & TECHNOLOGY
卷 8, 期 10, 页码 2617-2623出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cy00351c
关键词
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资金
- National Natural Science Foundation of China [21777044]
- National Key Research and Development Program [2016YFA0204200]
- China Postdoctoral Science Foundation [2015T8049]
- Fundamental Research Funds for the Central Universities [222201714061, 222201817009]
The photocatalytic activity of g-C3N4 was restricted by the fast charge recombination of photo-generated electrons and holes. In this work, a g-C3N4 metal-free composite modified with g-C3N4 quantum dots (CNQDs) (CNQDs/CN) was successfully prepared by a simple solvothermal method aiming to greatly promote the charge separation rate. The CNQDs/CN composite was confirmed by HRTEM and XPS measurements and exhibited outstanding photocatalytic activity in the degradation of organic pollutants represented by Rhodamine B. The enhanced photocatalytic performance of the CNQDs/CN composite can be ascribed to the effective charge separation and transfer across the interfaces between g-C3N4 and CNCtDs, which benefits from the excellent photoelectrochemical properties as well as the prolonged lifetime of charge carriers. The self-modification strategy provides a rational and interesting design idea to fabricate highly efficient photocatalysts.
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