期刊
ADVANCED ENERGY MATERIALS
卷 8, 期 21, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201800064
关键词
carbon black; large-scale energy storage; mechanical-chemical toughness; mulberry paper; PEDOT:PSS
类别
资金
- National Research Foundation of Korea (NRF) - Korea government (MSIP) [NRF-2016R1A2B3011473]
- R&D Convergence Program of MSIT (Ministry of Science and ICT)
- R&D Convergence Program of NST (National Research Council of Science & Technology) of Republic of Korea [CAP-13-01-KITECH]
- Korea Institute of Machinery and Materials [NK211B]
In response to the demand for flexible and sustainable energy storage devices that exhibit high electrochemical performance, a supercapacitor system is fabricated using mulberry tree-derived paper as a substrate and Poly(3,4-ethylenedioxythiophene)-poly( styrenesulfonate) (PEDOT:PSS) and carbon black as the active material. The mulberry paper-based supercapacitor system demonstrates high energy density of 29.8-39.8 Wh kg(-1) and power density of 2.8-13.9 kW kg(-1) with 90.7% retention of its initial capacity over 15 000 charge-discharge cycles. In addition, the mulberry tree fibers are known to have superior mechanical strength and toughness and the mulberry paper-based supercapacitor; as a result, exhibit high mechanical and chemical toughness; 99% of its initial capacity is retained after 100 repeated applications of bending strains, and twisting. 94% capacity retention is observed even after exposure to HCl and H2SO4 acid solutions. The fabrication methodology of the mulberry-based supercapacitor is highly scalable and could be stacked to increase the energy storage capacity, where operation of light-emitting diode lights with a drive voltage of 12 V integrated in a wearable device is demonstrated.
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