期刊
SMALL
卷 14, 期 29, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/smll.201800987
关键词
charge transport; electromagnetic energy conversion; graphene; relaxation; self-power
类别
资金
- National Natural Science Foundation of China [11774027, 51132002, 11574261, 11604237, 51072024, 51372282]
Electromagnetic energy radiation is becoming a health-killer of living bodies, especially around industrial transformer substation and electricity pylon. Harvesting, converting, and storing waste energy for recycling are considered the ideal ways to control electromagnetic radiation. However, heat-generation and temperature-rising with performance degradation remain big problems. Herein, graphene-silica xerogel is dissected hierarchically from functions to genes, thermally driven relaxation and charge transport, experimentally and theoretically, demonstrating a competitive synergy on energy conversion. A generic approach of material genes sequencing is proposed, tactfully transforming the negative effects of heat energy to superiority for switching self-powered and self-circulated electromagnetic devices, beneficial for waste energy harvesting, conversion, and storage. Graphene networks with well-sequencing genes (w = P-c/P-p > 0.2) can serve as nanogenerators, thermally promoting electromagnetic wave absorption by 250%, with broadened bandwidth covering the whole investigated frequency. This finding of nonionic energy conversion opens up an unexpected horizon for converting, storing, and reusing waste electromagnetic energy, providing the most promising way for governing electromagnetic pollution with self-powered and self-circulated electromagnetic devices.
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