4.8 Article

Polaronic behavior in a weak-coupling superconductor

出版社

NATL ACAD SCIENCES
DOI: 10.1073/pnas.1713916115

关键词

superconductivity; electronic structure; polaron; oxide interface

资金

  1. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-76SF00515]
  2. Gordon and Betty Moore Foundation's Emergent Phenomena in Quantum Systems Initiative [GBMF4415]
  3. University of Tennessee's Science Alliance Joint Directed Research and Development program
  4. Oak Ridge National Laboratory

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The nature of superconductivity in the dilute semiconductor SrTiO3 has remained an open question for more than 50 y. The extremely low carrier densities (10(18)-10(20) cm(-3)) at which superconductivity occurs suggest an unconventional origin of superconductivity outside of the adiabatic limit on which the Bardeen Cooper Schrieffer (BCS) and Migdal Eliashberg (ME) theories are based. We take advantage of a newly developed method for engineering band alignments at oxide interfaces and access the electronic structure of Nb-doped SrTiO3, using high-resolution tunneling spectroscopy. We observe strong coupling to the highest-energy longitudinal optic (LO) phonon branch and estimate the doping evolution of the dimensionless electron phonon interaction strength (lambda). Upon cooling below the superconducting transition temperature (T-c), we observe a single superconducting gap corresponding to the weak-coupling limit of BCS theory, indicating an order of magnitude smaller coupling (lambda(BCS) approximate to 0.1). These results suggest that despite the strong normal state interaction with electrons, the highest LO phonon does not provide a dominant contribution to pairing. They further demonstrate that SrTiO3 is an ideal system to probe superconductivity over a wide range of carrier density, adiabatic parameter, and electron phonon coupling strength.

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