期刊
NEW CARBON MATERIALS
卷 28, 期 1, 页码 66-70出版社
ELSEVIER
DOI: 10.1016/S1872-5805(13)60066-9
关键词
Carbon micro-spheres; Unpaired spins; Paramagnetism; Defects
资金
- National Natural Science Foundation of China [51072079]
- State Key Program for Basic Research [2010CB923402, 2012CB932304]
Interconnected carbon micro-spheres (CMSs) with diameters in the range of 3 similar to 5 mu m were synthesized by acetylene pyrolysis at 750 degrees C on a SiO2 substrate. The CMSs have a graphitic structure with many intrinsic defects. Results indicate that the CMSs show both diamagnetic and paramagnetic behavior. Intrinsic defects have magnetic moments with spin 1/2. Approximately every 1,000 carbon atoms contribute 1.1 mu(B) unpaired spins. The unpaired spins have no interactions with each other and show typical Curie-like paramagnetic behavior.
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