4.8 Article

Large Excitonic Reflectivity of Monolayer MoSe2 Encapsulated in Hexagonal Boron Nitride

期刊

PHYSICAL REVIEW LETTERS
卷 120, 期 3, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.120.037402

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资金

  1. DoD Vannevar Bush Faculty Fellowship [N00014-16-1-2825]
  2. AFOSR MURI [FA9550-12-1-0024, FA9550-17-1-0002]
  3. NSF [PHY-1506284, PHY-1125846, W911NF1520067]
  4. Gordon and Betty Moore Foundation
  5. Samsung Electronics

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We demonstrate that a single layer of MoSe2 encapsulated by hexagonal boron nitride can act as an electrically switchable mirror at cryogenic temperatures, reflecting up to 85% of incident light at the excitonic resonance. This high reflectance is a direct consequence of the excellent coherence properties of excitons in this atomically thin semiconductor. We show that the MoSe2 monolayer exhibits power-and wavelength-dependent nonlinearities that stem from exciton-based lattice heating in the case of continuous-wave excitation and exciton-exciton interactions when fast, pulsed laser excitation is used.

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