期刊
ORGANIC LETTERS
卷 20, 期 14, 页码 4341-4345出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.8b01791
关键词
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资金
- Agencia Estatal de Investigacion (AEI)/FEDER, UE [CTQ2016-75960-P]
- Severo Ochoa Excellence [SEV-2013-0319]
- Severo Ochoa Excellence (FPI predoctoral fellowship)
- European Research Council [321066]
- AGAUR [2017 SGR 1257]
- CERCA Program/Generalitat de Catalunya
Through the design of a second generation of more reactive 7-substituted 1,3,5-cycloheptatrienes, a room-temperature gold(I)-catalyzed retro-Buchner-cyclopropanation sequence and the first zinc(II)-catalyzed version of this process, which uses inexpensive ZnBr2 as catalyst, have been developed. This led to a broad-scope cyclopropanation of both activated and unactivated alkenes, including late-stage derivatization of biologically relevant compounds, and to the total synthesis of (+/-)-lactobacillic acid.
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